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毕业论文网 > 任务书 > 理工学类 > 应用物理 > 正文

BiVO4光电极的制备及其光电催化性能的研究任务书

 2020-04-29 19:05:13  

1. 毕业设计(论文)的内容和要求

随着科技的发展和社会的进步,人类面临着能源短缺和环境污染两大问题。

如何解决这些问题,实现能源和环境的可持续发展,成为人类亟待解决的议题。

光催化技术,从利用清洁能源太阳能的角度,实现氢能经济和人工光合作用,为这两大问题提供了终极解决途径。

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2. 参考文献

[1] D. K. Lee, K.-S. Choi. Enhancing long-term photostability of BiVO4 photoanodes for solar water splitting by tuning electrolyte composition. Nature Energy, 2018, 3(1), 53-60. [2] F. A. L. Laskowski, M. R. Nellist, J. Qiu, S. W. Boettcher. Metal Oxide/(oxy)hydroxide Overlayers as Hole Collectors and Oxygen-Evolution Catalysts on Water-Splitting Photoanodes. Journal of the American Chemical Society, 2018, [3] M. R. Huang, C. L. Li, L. Zhang, Q. Chen, Z. Zhen, Z. H. Li, H. W. Zhu. Twin Structure in BiVO4 Photoanodes Boosting Water Oxidation Performance through Enhanced Charge Separation and Transport. Adv Energy Mater, 2018, 8(32), [4] J. Zhu, F. Fan, R. Chen, H. An, Z. Feng, C. Li. Direct Imaging of Highly Anisotropic Photogenerated Charge Separations on Different Facets of a Single BiVO4 Photocatalyst. Angewandte Chemie-International Edition, 2015, 54(31), 9111-4. [5] F. Q. Zhou, J. C. Fan, Q. J. Xu, Y. L. Min. BiVO4 nanowires decorated with CdS nanoparticles as Z-scheme photocatalyst with enhanced H-2 generation. Applied Catalysis B-Environmental, 2017, 201(77-83. [6] M. Zhong, T. Hisatomi, Y. Kuang, J. Zhao, M. Liu, A. Iwase, Q. Jia, H. Nishiyama, T. Minegishi, M. Nakabayashi, N. Shibata, R. Niishiro, C. Katayama, H. Shibano, M. Katayama, A. Kudo, T. Yamada, K. Domen. Surface Modification of CoOx Loaded BiVO4 Photoanodes with Ultrathin p-Type NiO Layers for Improved Solar Water Oxidation. Journal of the American Chemical Society, 2015, 137(15), 5053-60. [7] W. Zhao, Y. Liu, Z. Wei, S. Yang, H. He, C. Sun. Fabrication of a novel p-n heterojunction photocatalyst n-BiVO4@p-MoS2 with core-shell structure and its excellent visible-light photocatalytic reduction and oxidation activities. Applied Catalysis B-Environmental, 2016, 185(242-52. [8] N. Tian, H. Huang, Y. He, Y. Guo, T. Zhang, Y. Zhang. Mediator-free direct Z-scheme photocatalytic system: BiVO4/g-C3N4 organic-inorganic hybrid photocatalyst with highly efficient visible-light-induced photocatalytic activity. Dalton Transactions, 2015, 44(9), 4297-307. [9] Y. Tang, R. Wang, Y. Yang, D. Yan, X. Xiang. Highly Enhanced Photoelectrochemical Water Oxidation Efficiency Based on Triadic Quantum Dot/Layered Double Hydroxide/BiVO4 Photoanodes. Acs Appl Mater Inter, 2016, 8(30), 19446-55. [10] J. Resasco, H. Zhang, N. Kornienko, N. Becknell, H. Lee, J. Guo, A. L. Briseno, P. Yang. TiO2/BiVO4 Nanowire Heterostructure Photoanodes Based on Type II Band Alignment. Acs Central Science, 2016, 2(2), 80-8. [11] Y. Pihosh, I. Turkevych, K. Mawatari, J. Uemura, Y. Kazoe, S. Kosar, K. Makita, T. Sugaya, T. Matsui, D. Fujita, M. Tosa, M. Kondo, T. Kitamori. Photocatalytic generation of hydrogen by core-shell WO3/BiVO4 nanorods with ultimate water splitting efficiency. Scientific Reports, 2015, 5( [12] H. Li, K. Yu, X. Lei, B. Guo, H. Fu, Z. Zhu. Hydrothermal Synthesis of Novel MoS2/BiVO4 Hetero-Nanoflowers with Enhanced Photocatalytic Activity and a Mechanism Investigation. Journal of Physical Chemistry C, 2015, 119(39), 22681-9. [13] H. Li, Y. Sun, B. Cai, S. Gan, D. Han, L. Niu, T. Wu. Hierarchically Z-scheme photocatalyst of Ag@AgCl decorated on BiVO4 (040) with enhancing photoelectrochemical and photocatalytic performance. Applied Catalysis B-Environmental, 2015, 170(206-14. [14] Y. Kuang, Q. Jia, H. Nishiyama, T. Yamada, A. Kudo, K. Domen. A Front-Illuminated Nanostructured Transparent BiVO4 Photoanode for 2% Efficient Water Splitting. Adv Energy Mater, 2016, 6(2), [15] H. J. Kong, D. H. Won, J. Kim, S. I. Woo. Sulfur-Doped g-C3N4/BiVO4 Composite Photocatalyst for Water Oxidation under Visible Light. Chemistry of Materials, 2016, 28(5), 1318-24.

3. 毕业设计(论文)进程安排

2018年12月-2019年1月 查找相关文献资料,了解实验的装置,相关的理论,写开题报告,开展初步的实验; 2019年2月-2019年4月 全面开展实验,具体包括样品的制备,数据的采集,数据的初步分析等; 2019年5月 毕业论文的撰写,毕业论文的答辩等

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